Well, it doesn't seem like any specific file is causing the issue; however, after it starts to get in too many textures, it will crash. I can get it to boot with a higher amount (but not all), and textures will show up in weird colors (i.e. the grass is blue instead of green).
Also, my framerate takes a pretty big nosedive, and the sound becomes extraordinarily choppy.
...One more thing to add that I don't feel like adding in since I just noticed it. >.> Some textures won't load at all (i.e. Lon Lon Ranch had a lot of white), so yeah. I believe it's a video plugin issue. I'll test different settings to see if I can resolve the problem.
EDIT
Ugh, no luck whatsoever. I can't seem to figure out what's causing the problem, but it only happens when so many textures are loaded in. Also, for some reason, the textures don't seem to cache, so loading takes a rather absurd amount of time.