If you ask me, you're probably better in the long run to either buy a new pc or upgrade your motherboard and processor, think about it, processors can cost only $50 or £30 (if you're british). motherboards can cost around the same... course you'd probably have to buy DDR ram too if you don't have any.
To sqeeze a few mhz out of your 666mhz (devil clock mhz

) seems rather pointless to me, but as they say, you need to overclock your fsb (front side bus), there may be an option for this in the Bios, just a warning though, your system could become unstable if you do this.
Hence why I say its rather pointless
Your ram speed won't really affect the speed of the processor, don't mess with that, it won't do you any good.
Good luck anyway!